Hi Jason,
"Officially", yes, it will need cal after any repair. Unofficially, The 2400s were pretty resilient to power supply fluctuations, you'll probably find it's pretty close to spec.
Why do you want to increase the capacitance on some of the caps? Those supplies were very well designed, if they wanted higher capacitance, they would have put in higher capacitance.
Don't forget that when you increase the capacitance you often also increase other parasitics, those can have unexpected affects. You'll also be changing the resonant points of the filters, which could easily lead to your low pass filter no longer rejecting some of the power supply noise.
I would strongly suggest not changing any of the values unless you have very good reason to do so and understand how it might affect the system.
73